Simultaneous And Stereoselective Formation Of Planar And Axial Chiralities In Enantiopure Sulfinyl Iron Diene Complexes

Document Type

Article

Publication Date

2-6-2003

Published In

Organic Letters

Abstract

Enantiopure (1Z,3E)-1-sulfinyl dienes bearing an o-dithianylphenyl group can be prepared and complexed with (bda)Fe(CO)(3) to afford the corresponding sulfinyl diene iron(0) tricarbonyl complexes. This diastereoselective complexation introduces planar and axial chirality simultaneously, with a high degree of facial selectivity as well as atropselectivity. Dynamic kinetic resolution is likely to be the origin of the atropselectivity.

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