Nonadiabatic Transitions In The Dynamics Of The NeICl Van Der Waals Complex

Document Type

Article

Publication Date

7-1-1989

Published In

Chemical Physics Letters

Abstract

Both electronic energy transfer and vibrational predissociation decay channels are observed following excitation of NeICl complexes to the β ion-pair state. Dispersed fluorescence is detected on the E→X transition as well as the D′→A′ and/or β→A transitions. The vibrational quantum number of the emitting level is reflected in the shape of the Franck-Condon envelope, while its electronic character is determined from the emission wavelength and profile. The relaxation pathways are found to depend on the initial vibrational excitation of the NeICl complex.

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